Study of Dyeing, Absorbency, Mechanical and Surface Properties on Chemical Treated Cotton Fabric

 

Jeyakodi  Moses J.1*,  Venkataraman V.K.2

1Associate Professor, Department of Applied Science, PSG College of Technology, Coimbatore 641 004, India

2Senior Grade Lecturer, Department of Chemistry and Applied Chemistry, PSG Polytechnic College, Coimbatore 641 004, India

*Corresponding Author E-mail: jj_moses2k2@yahoo.co.in

 

ABSTRACT:

Chemical treatment of cotton cellulose to alter its properties of the fibers without changing their fibrous form is a common practice nowadays in the textile industry.   In this paper cotton (woven and knitted) fabrics are selected and reacted with sodium hydroxide, morpholine, and cellulase enzyme.  The fabrics are then dyed by some selected dyes such as annatto, onion, pomegranate, indigo, myrobalan, bar berry (natural dyes); and reactive and sulphur dyes (synthetic) respectively and subsequently finished. These fabrics are then analyzed for k/s values, fastness properties, absorbency, water retention, wicking, mechanical and surface properties from KES-F.

 

KEYWORDS: Cotton  fabrics, Chemical treatment,  k/s values, wicking, KES-F.

 

 


INTRODUCTION:

Today cotton is the most used textile fiber in the world.  World textile fiber consumption in the end of 20th century was approximately 45 million tons.  Of this total, cotton represented approximately 20 million tons (1).  India holds the largest area of 8 m ha under cotton cultivation and ranked third in world’s cotton production, next to China and USA and second largest consumer of cotton (1, 2). Unlike synthetic fibres, cotton is a natural product (3) and  non-allergic since it doesn’t irritate sensitive skin or cause allergies.   Cotton has a high absorbency (4) rate and holds up to 27 times its own weight in water.   Cotton swells in a high humidity environment, in water and in concentrated solutions of certain acids, salts and bases (5).

 

Chemical treatment of cotton cellulose to alter physical properties of the fibers without changing their fibrous form is a common practice in the textile industry (6).  In the application of dyestuffs to cotton, several factors are considered as of prime importance (7-9). The importance of natural dyes has increased presently, with increased awareness about harmful effects of chemical dyes both in production and in its usage by human beings (10-12). This dye has the rare distinction of being a dye whose use can be traced back to antiquity and which continues to be as commonly used all over the world today as it is in the ancient times (13-16).            

 

This research work focuses on the treatment of cotton (woven and knitted) fabrics with sodium hydroxide, morpholine, and cellulase enzyme in order to improve its behaviour revealed by dyeing and finishing.  The cotton fabrics (treated and untreated) were dyed by some selected dyes such as annatto, onion, pomegranate, indigo, myrobalan, bar berry (natural dyes); and reactive  and sulphur dyes (synthetic) respectively and subsequently finished. These fabrics were then assessed for k/s values, fastness properties, absorbency, water retention, wicking, mechanical and surface properties from KES-F. 

 

EXPERIMENTAL:

Materials

Cotton (woven and knitted) fabrics with following specifications were used in this study.

 

Woven Fabric

Knitted fabric

Ends / Inch

Picks / Inch

GSM

Yarn  Count (Ne)

Yarn count (Ne)

GSM

Loop

length (mm)

Warp

Weft

 

84

 

94

146.1

 

27.1

 

26.1

 

27.5

 

136.9

2.6

 

 

Natural dyes [annatto (Bixa orellana), onion (Allium cepa), pomegranate (Punica granatum), indigo (Indigofera tinctoria), myrobalan (Terminalia chebula), bar berry (Berberis vulgaris)] and synthetic dyes [reactive dye  (reactive red HB – C.I. No. Red 24), and sulphur dye (sulphur black – C.I. No. sulphur Black 1)] used were in the commercial grade.  The commercial Super FX UltraSoft 2015 (Tirupur, India) was used for finishing on cotton fabrics.  The other chemicals mentioned elsewhere for this study were in AR grade.

 

Methods

Pretreatment on cotton (woven and knitted) fabrics

The cotton fabrics (woven and knitted) were pretreated (scouring and bleaching) as per the established technique (17, 18).

 

Sodium hydroxide treatment on cotton (woven and knitted) fabrics

The cotton fabrics (woven and knitted) were treated with sodium hydroxide of the concentration 15% (owm) for one hour at 85oC.

 

Morpholine treatment on cotton (woven and knitted) fabrics

The cotton fabrics (woven and knitted) were treated with aqueous solution of morpholine 40% for one hour at 40oC.

 

Cellulase enzyme treatment on cotton (woven and knitted) fabrics

The cotton fabrics (woven and knitted) were treated with Cellulase enzyme of the concentration 4.0% (owm) for one hour at 70oC.

 

Dyeing of cotton (woven and knitted) fabrics

The dyeability of cotton fabrics (woven and knitted) was investigated using natural and synthetic dyes. Dyeing was carried out at boil for two hours with a material to liquor ratio of 1:20 as per the established technique of dyeing for natural and synthetic dyes (18, 19). 

 

K/S analysis of the dyed cotton (woven and knitted) fabrics

Colorimetric data of natural and synthetic dyed cotton fabrics were determined by AATCC 135-1985 (20) technique using a Datacolor SF 600 plus spectrophotometer interfaced to a PC. Measurements were taken regarding colour presence, brightness, dullness and colour intensity with the specular component of the light excluded and the UV component included using illuminant D65 and 10° standard observer. Each fabric was folded once so as to give two thickness and average of five readings were taken each time. 

 

Color fastness analysis of the cotton (woven and knitted) fabrics

The natural and synthetic dyed samples were washed (AATCC, 2003) under condition IIIA of AATCC Test Method 124-2001 (21) to determine the color change effect of dyed fabrics. Light fastness tests (AATCC, 2003), were carried out according to AATCC Test Method 16 E-1998 (22) (2003). The samples were exposed to 5, 10 AFUs (AATCC Fading Unit) to determine the color change AATCC 16-1998 (23) (2003). AATCC standardized crock meter was used to determine the rubbing fastness (AATCC, 2003) of natural dyed fabrics under wet and dry condition to assess the color change and staining property AATCC 61-1996 (24) (2003).

 

Absorbency of cotton (woven and knitted) fabrics

Absorbency is the time taken for a water drop to penetrate into the silk material. The wettability of  cotton was determined (AATCC test method 79, 2010) (25) as per the established  technique and the average results were expressed in seconds.

 

Water retention in cotton (woven and knitted) fabrics

Water retaining capacity of cotton fabric was measured by the standard test method (AATCC 21-1978) (26).

 

Wicking behaviour of cotton (woven and knitted) fabrics

The wicking height of the cotton fabric was determined (27, 28). Fabric samples measuring 10 cm 2.5 cm were taken. Each of the sample pieces was clamped to a scale and held at a position such that the tip of the sample just touched the water taken in a beaker. 1% reactive dye (Reactive Red M8B, CI No.: Reactive Red 11) was added for tracking the movement of water. The height of water reached after five minutes was measured (29, 30).

 

Silicone softener finishing on cotton (woven and knitted) fabrics

The fabrics were finished with silicone softener (Super FX UltraSoft 2015) (Dosage: 5 – 10 gpl, pH: 5– 7, 30oC, 70 – 80% pick up, padded and dried at room temperature) and tested accordingly (31, 32).

 

Objective assessment on dyed and finished cotton (woven and knitted) fabrics by KES-F

The mechanical and surface properties of the dyed and finished woven and knitted cotton fabrics were assessed by Kawabata evaluation system (KES-F)  (33).

 

RESULTS AND DISCUSSION:

K/S values of dyed cotton (woven and knitted) fabrics

The K/S values of the dyes such as annatto, onion, pomogranate, indigo, myrobalan, barberry, reactive dye, and sulphur dye applied on cotton (woven and knitted) fabrics (sodium hydroxide treated, morpholine treated, cellulase treated and untreated) are given in Table 1.  From this table it is observed that woven cotton fabric shows overall high k/s values than the knitted cotton fabric.    The k/s value of sodium hydroxide treated cotton fabric is maximum when compared with morpholine treated, cellulase treated and untreated cotton fabrics.  The higher k/s value on the sodium hydroxide treated cotton fabric is influenced by the higher swelling action of sodium hydroxide followed by morpholine treatment and cellulase treatment.  Among the dyes applied on the cotton fabric (sodium hydroxide treated, morpholine treated, cellulase treated and untreated) there is only a marginal differences in the k/s values; however reactive dye shows the maximum k/s values. Even though the woven cotton fabric and knitted cotton fabric posses only a small differences in the k/s values for the dyes (annatto, onion, pomogranate, indigo, myrobalan, bar berry, reactive dye, and sulphur dye) applied on the cotton fabrics (sodium hydroxide treated, morpholine treated, cellulase treated and untreated); there is a uniform trend maintained in these values and the values of woven fabric give an edge over the knitted fabric.

 


 

 

 

Table 1. K/S values of dyed cotton (woven and  knitted) fabrics

S.

No.

Dyes

Colours obtained

K/S values of the dyed cotton fabric

Woven

Knitted

1

2

3

4

1

2

3

 4

1

Annatto

Orange

12.47

13.98

13.10

12.88

12.08

13.72

12.77

12.63

2

Onion

Orange Red

12.51

14.50

13.17

13.15

12.25

13.70

12.98

12.88

3

Pomogranate

Brown

12.64

14.47

13.52

13.35

12.18

13.76

12.84

12.70

4

Indigo

Blue

13.24

14.60

14.33

14.30

12.98

14.01

13.45

13.15

5

Myrobalan

Green

12.48

14.45

13.62

13.48

12.65

13.66

13.76

12.81

6

Bar berry

Yellow

12.75

14.54

13.41

13.40

12.65

13.95

13.32

13.02

7

Reactive Dye

Red

13.95

15.07

14.95

14.92

13.62

14.42

14.25

14.05

8

Sulphur Dye

Black

13.60

14.65

14.32

14.30

13.32

14.21

13.65

13.35

1.  Untreated cotton                          2.  Sodium hydroxide treated cotton

3.  Morpholine treated cotton           4.  Cellulase enzyme treated cotton

 

 


Washing fastness of the dyed cotton (woven and  knitted) fabrics

The washing fastness of the dyed (annatto, onion, pomogranate, indigo, myrobalan, bar berry, reactive dye, and sulphur dye) woven and knitted cotton fabrics are given in Table 2.  There is no significant improvement in the wash fastness of the woven and knitted cotton fabric (sodium hydroxide treated, morpholine treated, cellulase treated and untreated) dyed with annatto, onion, pomogranate, indigo, myrobalan, bar berry, reactive dye, and sulphur dyes.  However, the sodium hydroxide treated and dyed (annatto, onion, pomogranate, indigo, myrobalan, bar berry, reactive dye, and sulphur dye) cotton fabric (woven and knitted) shows improved wash fastness compared to the corresponding morpholine treated, cellulase treated and untreated cotton fabrics.  Among the dyes (annatto, onion, pomogranate, indigo, myrobalan, bar berry, reactive dye, and sulphur dye) applied on cotton fabric (woven and knitted) (sodium hydroxide treated, morpholine treated, cellulase treated and untreated) the reactive dyed one gives higher wash fastness over that of the other dyed ones (annatto, onion, pomogranate, indigo, myrobalan, bar berry, and sulphur dye). Even though the trend is followed similarly both in woven fabrics and knitted fabrics, the woven fabrics show marginal increase over the knitted dyed fabrics.

 


 

 

Table 2. Washing fastness of the dyed cotton (woven and  knitted)  fabrics

S.No.

Dyes

Washing fastness of the dyed fabric

Woven

Knitted

1

2

3

4

1

2

3

4

1

Annatto

3

3-4

3-4

3

3

3-4

3

3

2

Onion

3

4

3-4

3-4

2-3

3-4

3-4

3

3

Pomogranate

.3

3-4

3

3

.3

3

3

3

4

Indigo

3-4

4-5

4

4

3-4

4

4

4

5

Myrobalan

3

3-4

3-4

3-4

2-3

3-4

3-4

3

6

Bar berry

3

3-4

3

3

3

3

3-4

3-4

7

Reactive Dye

3-4

4-5

4-5

4

3-4

4-5

4

4

8

Sulphur Dye

3-4

4-5

4

4

3-4

4

4

4

1.  Untreated cotton                          2.  Sodium hydroxide treated cotton

3.  Morpholine treated cotton           4.  Cellulase enzyme treated cotton

 

 


Light fastness of the dyed cotton (woven and  knitted) fabrics

The light fastness of the dyed (annatto, onion, pomogranate, indigo, myrobalan, bar berry, reactive dye, and sulphur dye) woven and knitted cotton fabrics are given in Table 3.   From this table, it is seen that the overall light fastness of the woven and knitted cotton fabric (sodium hydroxide treated, morpholine treated, cellulase treated and untreated) dyed with annatto, onion, pomogranate, indigo, myrobalan, bar berry, reactive dye and sulphur dye is good (average 4-5).  The sodium hydroxide treated cotton fabric (woven and knitted) dyed with annatto, onion, pomogranate, indigo, myrobalan, bar berry, reactive dye, and sulphur dye shows higher light fastness values than the morpholine treated, cellulase treated and untreated cotton fabrics.  The high light fastness of the dyed (annatto, onion, pomogranate, indigo, myrobalan, bar berry, reactive dye, and sulphur dye) cotton fabric is influenced by sodium hydroxide treatment for more swelling thereby more dyeing reaction in cotton fabric (woven and knitted) followed by morpholine treatment, cellulase treatment and no treatment.  The reactive dye gives more light fastness value (average 5 – 6) when compared with all the other applied dyes (annatto, onion, pomogranate, indigo, myrobalan, bar berry, and sulphur dye)   (average 5) on cotton fabric (woven and knitted).  Similarly there is a uniform trend between woven fabric and knitted fabric for light fastness values on the treated (sodium hydroxide treated, morpholine treated, cellulase treated and untreated) and dyed (annatto, onion, pomogranate, indigo, myrobalan, bar berry, reactive dye, and sulphur dye) cotton fabric, however the woven fabric has an edge over the corresponding knitted fabric.

 


 

Table 3. Light fastness of the dyed cotton (woven and  knitted) fabrics

S.No.

Dyes

Light fastness of the dyed cotton fabric

Woven

Knitted

1

2

3

4

1

2

3

4

1

Annatto

4

5

4-5

4-5

3-4

4-5

4

4

2

Onion

4

5

5

4-5

3-4

4-5

4

4

3

Pomogranate

4

5

5

4

3-4

4-5

4-5

4

4

Indigo

4-5

5-6

5-6

5-6

4

5

5

4-5

5

Myrobalan

4

5-6

5

4-5

3-4

5

5

4-5

6

Bar berry

3-4

4-5

4-5

4

3-4

4-5

4

4

7

Reactive Dye

4-5

6

6

5-6

4

5-6

5-6

5

8

Sulphur Dye

5

6

5-6

5-6

4

5-6

5

5

1.  Untreated cotton                          2.  Sodium hydroxide treated cotton

3.  Morpholine treated cotton           4.  Cellulase enzyme treated cotton

 

 


Rubbing fastness of the dyed cotton (woven and  knitted) fabrics

The rubbing fastness both in wet and dry state of the dyed (annatto, onion, pomogranate, indigo, myrobalan, bar berry, reactive dye, and sulphur dye) woven and knitted cotton fabrics (sodium hydroxide treated, morpholine treated, cellulase treated and untreated) are given in Table 4.  Table 4 shows that the rubbing fastness in dry state is extremely good than that of wet state.  The reactive dyes show marginal high value of rubbing fastness than other dyes (annatto, onion, pomogranate, indigo, myrobalan, bar berry, and sulphur dye) applied on woven and knitted cotton fabrics in the dry state whereas in the corresponding wet state, as expected the rubbing fastness is in the poor form.   The sodium hydroxide treated cotton fabrics (woven and knitted) dyed with annatto, onion, pomogranate, indigo, myrobalan, bar berry, reactive dye, and sulphur dye show increased rubbing fastness values compared with those from cellulase and untreated fabrics.  The sodium hydroxide treatment increases the swelling in cotton fabrics thereby correspondingly increases the penetration of dyes also, hence the increased rubbing fastness value is obtained.  The average rubbing fastness values for the dyed (annatto, onion, pomogranate, indigo, myrobalan, bar berry, reactive dye, and sulphur dye) woven cotton fabric (sodium hydroxide treated, morpholine treated, cellulase treated and untreated) has an edge over the corresponding knitted fabric.

 


 

Table 4.  Rubbing fastness of the dyed cotton  (woven and  knitted)  fabrics

Dyes

Rubbing fastness of the dyed cotton fabric

woven

Knitted

1

2

3

4

1

2

3

4

Wet

Dry

Wet

Dry

Wet

Dry

Wet

Dry

Wet

Dry

Wet

Dry

Wet

Dry

Wet

Dry

Annatto

 

2

2

2-3

4

2-3

3-4

2-3

3

2

2

2-3

3-4

2-3

3-4

2

3

Onion

2

2-3

2-3

4

2-3

3-4

2

3

2

2-3

2-3

3-4

2

3

2

3

Pomogranate

2

2-3

2-3

3-4

2-3

3-4

2-3

3-4

1-2

2-3

2-3

3-4

2-3

3

2

3

Indigo

2

3

3

3-4

2-3

3-4

2

3

1-2

2-3

2-3

3

2

3

2

3

Myrobalan

2

2

2-3

3-4

2-3

3-4

2

3

1-2

2

2-3

3-4

2

3-4

2

3

Bar berry

2

2-3

2-3

4

2-3

3-4

2-3

3-4

2

2-3

2-3

4

2-3

4

2-3

4

React

ive Dye

2

3

3

4

3

3-4

3

3-4

2

2-3

2-3

4

2-3

4

2-3

4

Sulphur Dye

2

2-3

2-3

3-4

2-3

3

2

3

1-2

2-3

2-3

3

2

3

2

3

1.  Untreated cotton                          2.  Sodium hydroxide treated cotton

3.  Morpholine treated cotton           4.  Cellulase enzyme treated cotton

 

 


Stain resistance of the dyed cotton (woven and  knitted) fabrics

The stain resistance of the dyed (annatto, onion, pomogranate, indigo, myrobalan, bar berry, reactive dye, and sulphur dye)  woven and knitted cotton fabrics (sodium hydroxide treated, morpholine treated, cellulase treated and untreated) are given in Table 5.   From this table, it is seen that the stain resistance of synthetic dyes (reactive dye  and sulphur dye)  is more compared to those of natural dyes (annatto, onion, pomogranate, indigo, myrobalan, and bar berry)  applied on both woven and knitted cotton fabrics (sodium hydroxide treated, morpholine treated, cellulase treated and untreated).  Similarly, natural dyes (annatto, onion, pomogranate, indigo, myrobalan, and bar berry) also give good stain resistance on woven and knitted cotton fabrics  (sodium hydroxide treated, morpholine treated, cellulase treated and untreated) comparably with synthetic dyes.  In general, the stain resistance of all these dyes (annatto, onion, pomogranate, indigo, myrobalan, bar berry, reactive dye, and sulphur dye)  dyed on woven and knitted cotton fabrics is good (average 3 - 4).  The sodium hydroxide treated cotton fabrics (woven and knitted) show high stain resistance values than morpholine treated, cellulase treated and untreated dyed (annatto, onion, pomogranate, indigo, myrobalan, bar berry, reactive dye, and sulphur dye)  fabrics. The woven fabrics fabrics (sodium hydroxide treated, morpholine treated, cellulase treated and untreated) give marginal increase in stain resistance values over the corresponding knitted fabrics dyed with annatto, onion, pomogranate, indigo, myrobalan, bar berry, reactive dye, and sulphur dyes.

 


 

 

Table 5.  Stain resistance of the dyed cotton (woven and  knitted) fabrics

S.

No.

Dyes

Stain resistance of the dyed cotton fabrics

Woven

Knitted

1

2

3

4

1

2

3

 4

1

Annatto

3

4

3-4

3-4

2-3

3-4

3-4

3

2

Onion

2-3

4

3

3

2-3

3-4

3

3

3

Pomogranate

3

4

3-4

3-4

2-3

3-4

3

3

4

Indigo

3

4-5

4

3-4

3

4

3-4

3

5

Myrobalan

3-4

5

4

4

3

4

3-4

3-4

6

Bar berry

3

4

3-4

3-4

3

3-4

3-4

3

7

Reactive Dye

3-4

5

4

4

3-4

4

4

4

8

Sulphur Dye

3-4

4-5

4

4

3

4

3-4

3-4

1.  Untreated cotton                          2.  Sodium hydroxide treated cotton

3.  Morpholine treated cotton           4.  Cellulase enzyme treated cotton


 

 

 

Absorbency of  cotton  (woven and knitted) fabrics

The data of absorbency of cotton (woven and knitted) fabrics (sodium hydroxide treated, morpholine treated, cellulase treated and untreated) dyed with annatto, onion, pomogranate, indigo, myrobalan, barberry, reactive dye (H), and sulphur dye is given in Table 6.  It is seen from this table that the overall absorbency exhibited by woven cotton fabric is more than that of knitted cotton fabric.   The absorbency of treated cotton (sodium hydroxide, morpholine, and cellulase) fabrics is substantial when compared with the untreated one.  Among the treated cotton (sodium hydroxide, morpholine, and cellulase) fabrics the sodium hydroxide treated cotton fabric shows maximum absorbency followed by morpholine treated and cellulase treated cotton fabrics.  Between the dyed (annatto, onion, pomogranate, indigo, myrobalan, bar berry, reactive dye (H), and sulphur dyes) cotton fabrics (sodium hydroxide treated, morpholine treated, cellulase treated and untreated) only a marginal difference in the absorbency is noted, however the reactive dyed cotton fabrics show maximum absorbency value.  The trend is followed in the similar way for both the woven cotton fabrics and knitted cotton fabrics. 

                     


 

 

Table 6.  Absorbency of  cotton  (woven and knitted) fabrics

S.

No.

Dyes

Drop absorbency (seconds) of the dyed cotton fabrics

Woven

Knitted

1

2

3

4

1

2

3

4

1

Annatto

25

10

13

16

27

14

16

18

2

Onion

25

10

12

15

26

14

16

18

3

Pomogranate

24

10

12

14

26

12

15

16

4

Indigo

28

12

15

19

30

15

18

22

5

Myrobalan

24

11

12

15

26

13

16

18

6

Barberry

23

9

11

13

25

12

15

16

7

Reactive Dye

22

9

10

12

25

11

13

14

8

Sulphur Dye

28

14

17

20

31

16

19

24

1.  Untreated cotton                                           2.  Sodium hydroxide treated cotton

3.  Morpholine treated cotton           4.  Cellulase enzyme treated cotton

 

 


Water retention in cotton (woven and knitted) fabrics

The data of water retention of cotton (woven and knitted) fabrics (sodium hydroxide treated, morpholine treated, cellulase treated and untreated) dyed with annatto, onion, pomogranate, indigo, myrobalan, barberry, reactive dye (H), and sulphur dye is given in Table 7.  Table 7 reveals that the water retention behaviour is due to the presence of hydrophilic groups present in the polymers of the selected fabrics and also by the treatment using sodium hydroxide, morpholine,  and cellulase.  The amount of water retained by the fiber mass increases with an increase in the hydrophilic tendency of the fiber due to the corresponding treatments.  The sodium hydroxide treated fabric shows maximum water retaining behaviour followed by the morpholine treatment and cellulase enzyme treatment.  From the Table 7, it is also observed that the woven  fabric gives relatively more water retention behaviour than that of the knitted fabric. The reactive dyed materials show the maximum water retention followed by bar berry, myrobalan, annatto, onion, pomogranate, indigo, and sulphur dyed textiles.

 


 

 

Table 7.  Water retention in cotton  (woven and knitted) fabrics

S.

No.

Dyes

Water retention (%) of the dyed cotton fabrics

Woven

Knitted

1

2

3

4

1

2

3

4

1

Annatto

345                                             345

354                                             345

350                                             345

348                                             345

342                                             345

350                                             345

346                                             345

345                                             345

2

Onion

343

352

348

346

340

349

345

343

3

Pomogranate

342

353

349

346

338

350

346

344

4

Indigo

340

349

345

342

337

346

342

339

5

Myrobalan

349

361

357

354

346

358

355

351

6

Barberry

350

363

358

355

347

360

356

352

7

Reactive Dye

   352                                          345

365

360

   356                                          345

   350                                          345

362

358

   353                                          345

8

Sulphur Dye

338

350

345

342

335

347

342

339

 

 


 

Wicking of  cotton  (woven and knitted) fabrics                         

The data of wicking behaviour of cotton (woven and knitted) fabrics (sodium hydroxide treated, morpholine treated, cellulase treated and untreated) dyed with   annatto, onion, pomogranate, indigo, myrobalan, barberry, reactive dye  and sulphur dyes are given in Table 8.  From Table 8, it is clear that the wicking behaviour of all the samples is good, however woven fabrics show some edge over the knitted fabrics.   The wicking behaviour of sodium hydroxide treated cotton fabric is significantly high compared with those of untreated cotton fabric.  Among the treated cotton fabrics the sodium hydroxide treatment influences more on the wicking behaviour followed by morpholine treatment and cellulase treatment. The differences in the wicking behaviour of the dyed (annatto, onion, pomogranate, indigo, myrobalan, barberry, reactive dye, and sulphur dye) cotton fabric is only marginal.  However, the reactive dyed cotton fabric shows the high wicking value when compared with the other dyed cotton fabrics.  All the data are comparable and similar between the woven and knitted dyed cotton fabrics.

 


 

 

Table 8.  Wicking of  cotton  (woven and knitted) fabrics

S.

No.

Dyes

Wicking  (cm) of dyed cotton fabrics

Woven

Knitted

1

2

3

4

1

2

3

4

1

Annatto

8

15

14

12

7

14

11

10

2

Onion

8

16

14

13

7

14

12

11

3

Pomogranate

8

16

15

13

7

13

12

11

4

Indigo

7

15

13

12

5

12

11

10

5

Myrobalan

8

16

14

13

7

14

12

11

6

Bar berry

8

19

17

14

8

16

14

12

7

Reactive Dye

9

17

16

13

8

15

14

11

8

Sulphur Dye

6

14

12

11

5

11

10

09

1.  Untreated cotton                          2.  Sodium hydroxide treated cotton

3.  Morpholine treated cotton           4.  Cellulase enzyme treated cotton

 

 


Mechanical and surface properties from KES-F

The mechanical and surface properties of the dyed and finished cotton fabrics (woven and knitted) were objectively assessed by Kawabata evaluation system (KES-F). The primary hand value (PHV) (of both woven and knitted fabrics), bending length (of only woven fabric) fabrics, and crease recovery (of only woven fabric) of the dyed and finished cotton fabrics were carried out by this system and data are presented in Tables 9a and 9b, Table 2 and Table 3 respectively.

 

Primary hand value (PHV) of dyed and finished cotton (woven and knitted) fabrics

                The parameters evaluated from KES-F of dyed and finished cotton fabrics for the primary hand value in terms of smoothness, stiffness and fullness of woven and knitted fabrics are given in Tables 9a and 9b respectively.  From these Tables (9a and 9b) it is seen that the smoothness is observed more on the dyed and finished sodium hydroxide treated [2] cotton fabric followed by morpholine treated [3], enzyme treated [4] and untreated [1] cotton fabrics respectively.  The undyed / unfinished untreated [UT] cotton fabrics show very low smoothness values compared to the above mentioned treated fabrics.  The dyed fabrics [F1 / 1,2,3, 4] when finished [F2] with the finishing agent - Super FX UltraSoft 2015, the smoothness is considerably increased in all these cases [1,2,3,4].  The increased smoothness values on the dyed and finished cotton fabrics [F1, F2 / 1,2,3,4] compared to the untreated unfinished cotton fabrics [UT] are due to the good application of dyeing and finishing as promoted by good treatments [2,3,4].  Among the dyes, the differences in smoothness values on the cotton fabrics [UT, F1, F2 / 1,2,3,4] are only marginal.  Tables 1a and 1b also reveal that the stiffness of the fabrics is reduced due to the sodium hydroxide treatment, morphology treatment and enzyme treatment followed by dyeing and finishing.  Compared to all treated [F1, F2 / 2,3,4] and untreated [UT, and  F1, F2 / 1] fabrics the sodium hydroxide treated cotton fabrics show reduced stiffness, this is due to the good flexibility generated by sodium hydroxide; followed by morpholine treatment, enzyme treatment and untreated dyed and finished cotton fabrics.  The fullness is maximum on the sodium hydroxide treated cotton fabrics followed by morpholine treated, enzyme treated and untreated fabrics.  In general, the primary hand value is maximum for the sodium hydroxide treated [2] fabrics followed by morpholine treated [3], enzyme treated [4] and  untreated [UT, 1] dyed [F1]  and finished [F2] woven and knitted cotton fabrics (Table 1a and 1b).


 

 

 

 

Table 9a.    Primary hand value (PHV) of dyed and finished woven  cotton fabric

S.No.

Dyes

PHV of woven  cotton fabric

UT

1

2

3

4

F1

F2

F1

F2

F1

F2

F1

F2

 

1

2

3

4

5

6

7

8

9

Smoothness :

Undyed

Annatto

Onion

Pomogranate

 Indigo

Myrobalan

Bar berry

Reactive Dye

Sulphur Dye

 

2.7

2.9

2.8

2.8

2.7

2.8

2.8

3.2

2.3

 

5.0

5.4

5.3

5.3

5.2

5.2

5.3

5.7

4.9

 

5.4

5.8

5.5

5.5

5.5

5.5

5.6

6.0

5.3

 

7.3

7.5

7.4

7.6

7.4

7.6

7.7

7.7

7.5

 

7.8

7.9

7.6

7.7

7.6

7.7

7.9

7.8

7.6

 

6.6

6.7

6.6

6.8

6.7

6.8

6.9

6.8

6.6

 

6.7

6.8

6.7

7.0

6.8

6.9

7.1

7.0

6.8

 

6.4

6.5

6.5

6.6

6.5

6.5

6.7

6.6

6.4

 

6.5

6.6

6.6

6.7

6.7

6.6

6.8

6.7

6.5

 

1

2

3

4

5

6

7

8

9

Stiffness :

Undyed

Annatto

Onion

Pomogranate

Indigo

Myrobalan

Bar berry

Reactive Dye

Sulphur Dye

 

5.0

4.8

4.7

4.8

4.8

4.5

4.8

4.7

4.9

 

4.9

4.8

4.8

4.8

4.9

4.8

4.8

4.6

4.9

 

4.6

4.5

4.5

4.5

4.6

4.5

4.5

4.2

4.6

 

4.6

4.5

4.5

4.5

4.6

4.5

4.5

4.3

4.6

 

4.3

4.2

4.2

4.2

4.4

4.2

4.2

3.9

43

 

4.7

4.6

4.6

4.6

4.7

4.6

4.6

4.4

4.7

 

4.4

4.3

4.3

4.3

4.5

4.3

4.3

4.0

4.4

 

4.8

4.7

4.7

4.7

4.8

4.7

4.7

4.5

4.8

 

4.5

4.4

4.4

4.4

4.5

4.4

4.4

4.1

4.5

 

1

2

3

4

5

6

7

8

9

Fullness :

Undyed

Annatto

Onion

Pomogranate

Indigo

Myrobalan

Bar berry

Reactive Dye

Sulphur Dye

 

4.8

4.9

4.9

4.8

4.8

4.8

4.9

5.0

4.8

 

7.7

8.3

8.3

8.1

8.2

8.3

8.3

8.5

8.2

 

8.2

8.7

8.5

8.5

8.5

8.4

8.6

8.8

8.5

 

9.4

9.9

9.6

9.5

9.5

9.4

9.5

9.9

9.6

 

9.7

10.7

10.6

10.4

10.5

10.4

10.5

10.8

10.4

 

8.3

9.2

9.1

9.0

9.0

9.0

9.1

9.2

9.0

 

8.5

9.5

9.4

9.4

9.3

9.4

9.4

9.5

9.4

 

8.1

9.0

8.9

8.8

8.8

8.8

8.9

9.0

8.8

 

8.4

9.4

9.3

9.3

9.2

9.3

9.3

9.4

9.3

UT à undyed / unfinished / untreated cotton       1.  Untreated cotton       2.  Sodium hydroxide treated  cotton  

3.    Morpholine treated cotton    4.  Cellulase enzyme treated cotton

 

 

Table 9b.    Primary hand value (PHV)  of dyed and finished knitted  cotton fabric

S.No.

Dyed Samples

PHV of  knitted  cotton fabric

UT

1

2

3

4

F1

F2

F1

F2

F1

F2

F1

F2

 

1

2

3

4

5

6

7

8

9

Smoothness :

Undyed

Annatto

Onion

Pomogranate

 Indigo

Myrobalan

Bar berry

Reactive Dye

Sulphur Dye

 

2.4

2.8

2.7

2.6

2.7

2.6

2.8

3.1

2.5

 

4.8

5.2

5.1

4.9

5.0

4.9

5.1

5.5

4.8

 

5.2

5.6

5.4

5.3

5.4

5.3

5.5

5.9

5.3

 

6.8

7.1

6.9

6.7

6.6

6.6

6.7

7.0

6.9

 

7.1

7.3

7.2

7.2

7.3

7.3

7.4

7.5

7.2

 

6.2

6.6

6.5

6.3

6.4

6.3

6.4

6.6

6.3

 

6.3

6.7

6.7

6.6

6.6

6.5

6.5

6.7

6.4

 

5.9

6.2

6.2

6.0

6.1

6.0

6.2

6.4

5.9

 

6.2

6.4

6.5

6.3

6.4

6.3

6.4

6.6

6.3

 

1

2

3

4

5

6

7

8

9

Stiffness :

Undyed

Annatto

Onion

Pomogranate

Indigo

Myrobalan

Bar berry

Reactive Dye

Sulphur Dye

 

4.8

4.7

4.6

4.7

4.7

4.6

4.6

4.6

4.8

 

4.7

4.6

4.7

4.8

4.8

4.7

4.7

4.5

4.8

 

4.5

4.4

4.4

4.4

4.5

4.5

4.4

4.1

4.5

 

4.4

4.3

4.4

4.5

4.5

4.4

4.4

4.2

4.5

 

4.2

4.1

4.2

4.1

4.2

4.2

4.1

3.8

4.2

 

4.5

4.4

4.5

4.6

4.6

4.5

4.5

4.3

4.6

 

4.3

4.2

4.3

4.2

4.3

4.3

4.2

3.9

4.3

 

4.6

4.5

4.6

4.7

4.7

4.6

4.6

4.4

4.7

 

4.4

4.3

4.3

4.3

4.4

4.4

4.3

4.0

4.4

 

1

2

3

4

5

6

7

8

9

Fullness :

Undyed

Annatto

Onion

Pomogranate

Indigo

Myrobalan

Bar berry

Reactive Dye

Sulphur Dye

 

4.6

4.7

4.9

4.8

4.8

4.9

4.8

4.9

4.7

 

7.4

8.1

8.1

8.1

8.0

8.0

8.1

8.4

8.1

 

7.9

8.6

8.5

8.4

8.4

8.5

8.5

8.7

8.4

 

8.4

8.9

8.8

8.9

8.8

8.9

8.9

9.0

8.9

 

8.7

9.4

9.3

9.3

9.2

9.3

9.4

9.5

9.2

 

7.9

8.7

8.6

8.7

8.6

8.6

8.7

8.9

8.6

 

8.3

9.0

9.0

8.9

8.8

8.9

8.9

9.0

8.8

 

7.7

8.4

8.4

8.4

8.3

8.3

8.4

8.7

8.4

 

8.1

8.8

8.7

8.6

8.6

8.7

8.7

8.8

8.6

UT à undyed / unfinished / untreated cotton      1.  Untreated cotton    2.  Sodium hydroxide treated  cotton  

3.    Morpholine treated cotton    4.  Cellulase enzyme treated cotton


 

Bending length of dyed and finished woven cotton fabric

The values of the bending length of untreated [UT, 1] and treated [sodium hydroxide, morpholine and enzyme] dyed and finished woven cotton fabrics are given in Table 10.  From this table it is given as the data of the bending length both in warp and weft directions respectively of cotton fabric treated with sodium hydroxide, morpholine and enzyme followed by dyeing and finishing.   It is evident from the Table 10 that bending length both in warp and weft directions of dyed [F1] and finished [F2] cotton fabric treated with sodium hydroxide [2]  is least followed by morpholine treated [3], enzyme treated [4] and untreated [1] cotton fabrics respectively.  The undyed / unfinished untreated [UT] cotton fabric shows the maximum bending length (warp and weft) which is periodically reduced after the treatments such as enzyme, morpholine and sodium hydroxide and subsequent dyeing and finishing.  These treatments reduce the bending lengths on the cotton fabrics and sodium hydroxide treatment tops the list in this reduction followed by morpholine and enzyme treatments.  Dyeing and finishing also further enhances the reduction in bending lengths on all these fabrics.  There is no much influences in the differences of bending length due to the change of dyes (Annatto, Onion, Pomogranate, Indigo,  Myrobalan,  Bar berry,  Reactive Dye and  Sulphur dye).  The warp directions have marginally more bending length values in all these woven cotton fabrics.

                                                                                                       


 

Table  10.    Bending length of  dyed and finished woven cotton fabric

S.No.

Dyes

Bending length (mm) of woven cotton fabric

Warp (Cw)

UT

1

2

3

4

F1

F2

F1

F2

F1

F2

F1

F2

1

2

3

4

5

6

7

8

9

Undyed

Annatto

Onion

Pomogranate

Indigo

Myrobalan

Bar berry

Reactive Dye

Sulphur Dye

10.8

10.3

10.4

10.3

10.4

10.4

10.3

10.4

10.4

9.6

9.5

9.4

9.5

9.5

9.4

9.4

9.3

9.2

9.4

9.3

9.3

9.2

9.3

9.3

9.4

9.2

9.3

9.0

8.9

8.8

8.9

8.9

8.8

8.8

8.7

8.6

8.8

8.6

8.7

8.6

8.7

8.7

8.7

8.6

8.5

9.2

9.1

9.0

9.1

9.1

9.0

9.0

8.9

8.8

9.0

8.8

8.9

8.8

8.9

8.9

8.9

8.8

8.7

9.4

9.3

9.2

9.3

9.3

9.2

9.2

9.1

9.0

9.2

9.0

9.1

9.0

9.1

9.1

9.1

9.0

8.9

 

 

Bending length (mm) of woven cotton fabric

Weft (Cf)

 

 

 

 

1

2

3

4

UT

F1

F2

F1

F2

F1

F2

F1

F2

1

2

3

4

5

6

7

8

9

Undyed

Annatto

Onion

Pomogranate

Indigo

Myrobalan

Bar berry

Reactive Dye

Sulphur Dye

10.6

10.2

10.2

10.2

10.2

10.2

10.1

10.1

10.3

9.4

9.3

9.2

9.3

9.3

9.3

9.2

9.1

9.1

9.2

9.1

9.1

9.1

9.2

9.1

9.1

9.0

9.2

8.8

8.7

8.6

8.7

8.7

8.7

8.6

8.5

8.5

8.6

8.5

8.5

8.5

8.6

8.5

8.5

8.3

8.4

9.0

8.9

8.8

8.9

8.9

8.9

8.8

8.7

8.7

8.8

8.7

8.7

8.7

8.8

8.7

8.7

8.6

8.7

9.2

9.1

9.0

9.1

9.1

9.1

9.0

8.9

8.9

9.0

8.9

8.9

8.9

9.0

8.9

8.9

8.8

9.0

UT à undyed / unfinished / untreated cotton    1.  Untreated cotton        2.  Sodium hydroxide treated  cotton  

3.    Morpholine treated cotton    4.  Cellulase enzyme treated cotton

 


 

Crease recovery (o) of dyed and finished woven cotton fabric

The data of the crease recovery both in warp and weft directions of dyed and finished woven cotton fabric treated with sodium hydroxide, morpholine and enzyme are given in Table 11.  From this table, it is clearly seen that the crease recovery both in warp and weft directions of dyed [F1] and finished [F2] cotton fabric treated with sodium hydroxide [2] is minimum compared to morpholine treated [3], enzyme treated [4] and untreated cotton fabrics [1] respectively.  The undyed / unfinished untreated [UT] cotton fabric shows the maximum  crease recovery (warp and weft) which is subsequently reduced after the treatments such as enzyme, morpholine and sodium hydroxide and subsequent dyeing and finishing.  These treatments reduce the crease recovery on the cotton fabrics and sodium hydroxide treatment tops the list in this reduction followed by morpholine and enzyme treatments.  Dyeing and finishing also further enhances the reduction in crease recovery on all these fabrics.  The various dyes  (Annatto, Onion, Pomogranate, Indigo,  Myrobalan,  Bar berry,  Reactive Dye and  Sulphur dye).  do not give much influences in the differences of crease recovery.  The weft directions have marginally more crease recovery values than those in warp directions in all these woven cotton fabrics.

 

 


Table 11.  Crease recovery (o) of dyed and finished woven cotton fabric

S.No.

Dyes

Crease recovery  (o) of woven cotton fabric

Warp (Cw)

 

1

2

3

4

UT

F1

F2

F1

F2

F1

F2

F1

F2

1

2

3

4

5

6

7

8

9

Undyed

Annatto

Onion

Pomogranate

Indigo

Myrobalan

Bar berry

Reactive Dye

Sulphur Dye

112

109

109

110

110

110

109

104

111

109

103

105

106

106

105

104

100

107

107

99

99

100

100

100

98

96

102

99

94

95

96

97

95

94

91

96

96

89

90

89

91

91

88

87

92

104

98

99

101

101

99

98

94

100

100

93

94

94

95

95

92

91

96

107

101

103

104

104

103

101

97

104

104

96

97

97

98

98

95

94

99

 

 

Crease recovery  (o) of woven cotton fabric

Weft (Cf)

 

 

 

UT

1

2

3

4

F1

F2

F1

F2

F1

F2

F1

F2

1

2

3

4

5

6

7

8

9

Undyed

Annatto

Onion

Pomogranate

Indigo

Myrobalan

Bar berry

Reactive Dye

Sulphur Dye

114

111

111

111

112

112

111

105

113

112

104

107

108

108

108

106

104

109

110

102

104

103

104

103

103

100

105

105

97

100

101

102

101

99

97

100

103

95

97

96

97

96

96

94

97

108

100

103

104

104

104

102

100

104

106

98

100

99

100

99

99

96

100

110

102

105

106

106

106

104

102

107

108

100

102

101

102

101

101

98

103

UT à undyed / unfinished / untreated cotton    1.  Untreated cotton      2.  Sodium hydroxide treated  cotton  

3.    Morpholine treated cotton    4.  Cellulase enzyme treated cotton

 

 


CONCLUSION:

The conclusions drawn from the study are summarized below:

The K/S values of the dyes such as annatto, onion, pomogranate, indigo, myrobalan, barberry, reactive dye, and sulphur dye applied on cotton (woven and knitted) fabrics (sodium hydroxide treated, morpholine treated, cellulase treated and untreated) are good.  The sodium hydroxide treated cotton fabrics show maximum colour data  followed by morpholine treated and cellulase enzyme treated cotton fabrics. The fastness properties (wash, light, rubbing and stain resistance) of the dyed (annatto, onion, pomogranate, indigo, myrobalan, bar berry, reactive dye and sulphur dye) woven and knitted cotton fabrics (sodium hydroxide treated, morpholine treated, cellulase treated and untreated)  are good.  In general, the overall fastness properties are more in sodium hydroxide treated cotton fabrics followed by morpholine treated and cellulase enzyme treated cotton fabrics. The absorbency is good in both cotton (woven and knitted) fabrics (sodium hydroxide treated, morpholine treated, cellulase treated and untreated).  However the woven fabric gives increased absorption than the knitted fabric.  The water retention character is more in the woven cotton fabric than the knitted cotton fabric. As the absorption and water retention behaviour are more, obviously the wicking value is also good in both the type of fabrics, however the woven fabrics show more wicking behaviour compared to the knitted cotton fabric.

                The primary hand value such as smoothness, stiffness and fullness is good in sodium hydroxide treated, morpholine treated, enzyme treated woven and knitted cotton fabrics respectively.  Smoothness is observed more on the dyed and finished sodium hydroxide treated cotton fabric followed by morpholine treated, enzyme treated and untreated cotton fabrics respectively. The sodium hydroxide treated cotton fabrics have reduced stiffness due to the generation of good flexibility; followed by morpholine treatment, enzyme treatment and untreated dyed and finished cotton fabrics. The fullness is also maximum on the sodium hydroxide treated cotton fabrics followed by morpholine treated, enzyme treated and untreated fabrics.  In general, the primary hand value is maximum for the sodium hydroxide treated fabrics followed by morpholine treated, enzyme treated and  untreated dyed  and finished woven and knitted cotton fabrics. 

               

The bending length in both warp and weft directions of dyed and finished woven cotton fabric is good in sodium hydroxide treated one with  least value followed by morpholine treated, enzyme treated and untreated fabrics respectively.  The trend is common in both warp and weft directions, however the warp materials have an edge over the weft materials for the bending length. The crease recovery in both warp and weft directions of dyed and finished woven cotton fabric treated with sodium hydroxide is minimum compared to morpholine treated, enzyme treated  and untreated cotton fabric  respectively revealed the good effect of sodium hydroxide.  The trend is common in both warp and weft directions, however the weft materials have a little edge over the warp materials for the crease recovery.  

 

ACKNOWLEDGEMENT:

The authors wish to thank the Management and the Principal, PSG College of Technology, Coimbatore for given the permission and providing the necessary infrastructure. Thanks are also due to The Head, Department of Applied Science for the kind help in department laboratory supports.

 

REFERENCES:

1.        Lawrence Shaw H,  1998, Cotton’s Importance in the Textile Industry [Symposium], Lima, Peru.

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Received on 26.09.2015         Modified on 13.10.2015

Accepted on 16.10.2015         © AJRC All right reserved

Asian J. Research Chem. 8(11): November 2015; Page 664-674

DOI: 10.5958/0974-4150.2015.00107.8